Nanomechanical method to gauge emission quantum yield applied to nitrogen-vacancy centers in nanodiamond
We present a technique to nanomechanically vary the distance between a fluorescent source and a mirror, thereby varying the local density of optical states at the source position. Our method can, therefore, serve to measure the quantum efficiency of fluorophores. Application of our technique to nitrogen-vacancy defects in diamond nanocrystals shows that their quantum yield can significantly differ from unity. Relying on a lateral scanning mechanism with shear-force probe-sample distance control our technique is straightforwardly implemented in most state-of-the-art near-field microscopes.
|Reviewer||E. Verhagen (Ewold)|
|Journal||Appl. Phys. Lett.|
Frimmer, M, Mohtashami, A, & Koenderink, A.F. (2013). Nanomechanical method to gauge emission quantum yield applied to nitrogen-vacancy centers in nanodiamond. Appl. Phys. Lett., 102(12, Article number: 121105), 1–7. doi:10.1063/1.4798327