Cathodoluminescence spectroscopy (CL) allows characterizing light emission in bulk and nanostructured materials and is a key tool in fields ranging from materials science to nanophotonics. Previously, CL measurements focused on the spectral content and angular distribution of emission, while the polarization was not fully determined. Here we demonstrate a technique to access the full polarization state of the cathodoluminescence emission, that is the Stokes parameters as a function of the emission angle. Using this technique, we measure the emission of metallic bullseye nanostructures and show that the handedness of the structure as well as nanoscale changes in excitation position induce large changes in polarization ellipticity and helicity. Furthermore, by exploiting the ability of polarimetry to distinguish polarized from unpolarized light, we quantify the contributions of different types of coherent and incoherent radiation to the emission of a gold surface, silicon and gallium arsenide bulk semiconductors. This technique paves the way for in-depth analysis of the emission mechanisms of nanostructured devices as well as macroscopic media.

Additional Metadata
Publisher ACS
Reviewer L. Kuipers
Persistent URL dx.doi.org/10.1021/acsphotonics.5b00596
Journal ACS Photonics
Citation
Osorio, C.I, Coenen, T, Brenny, B.J.M, Polman, A, & Koenderink, A.F. (2016). Angle-resolved cathodoluminescence imaging polarimetry. ACS Photonics, 3(1), 147–154. doi:10.1021/acsphotonics.5b00596